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Homogenous reduced moment in a gapful scalar chiral kagome antiferromagnet

Authors :
Scheie, A.
Dasgupta, S.
Sanders, M.
Sakai, A.
Matsumoto, Y.
Prisk, T. R.
Nakatsuji, S.
Cava, R. J.
Broholm, C.
Source :
Phys. Rev. B 100, 024414 (2019)
Publication Year :
2019

Abstract

We present present a quantitative experimental investigation of the scalar chiral magnetic order with in $\rm{Nd_3Sb_3Mg_2O_{14}}$. Static magnetization reveals a net ferromagnetic ground state, and inelastic neutron scattering from the hyperfine coupled nuclear spin reveals a local ordered moment of 1.76(6) $\mu_B$, just 61(2)% of the saturated moment size. The experiments exclude static disorder as the source of the reduced moment. A 38(1) $\mu$eV gap in the magnetic excitation spectrum inferred from heat capacity rules out thermal fluctuations and suggests a multipolar explanation for the moment reduction. We compare $\rm{Nd_3Sb_3Mg_2O_{14}}$ to Nd pyrochlores and show that it is close to a moment fragmented state.<br />Comment: 5 pages, 4 figures, 3 pages supplemental information

Details

Database :
arXiv
Journal :
Phys. Rev. B 100, 024414 (2019)
Publication Type :
Report
Accession number :
edsarx.1904.11779
Document Type :
Working Paper
Full Text :
https://doi.org/10.1103/PhysRevB.100.024414