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Observation of semi-localized dispersive states in the strongly correlated electron-doped ferromagnet Eu$_{1-x}$Gd$_{x}$O

Authors :
Shai, Daniel E.
Fischer, Mark H.
Melville, Alex J.
Monkman, Eric J.
Harter, John W.
Shen, Dawei
Schlom, Darrell G.
Lawler, Michael J.
Kim, Eun-Ah
Shen, Kyle M.
Source :
Phys. Rev. B 94, 195102 (2016)
Publication Year :
2016

Abstract

Chemical substitution plays a key role in controlling the electronic and magnetic properties of complex materials. For instance, in EuO, carrier doping can induce a spin-polarized metallic state, colossal magnetoresistance, and significantly enhance the Curie temperature. Here, we employ a combination of molecular-beam epitaxy, angle-resolved photoemission spectroscopy, and an effective model calculation to investigate and understand how semi-localized states evolve in lightly electron doped Eu$_{1-x}$Gd$_{x}$O above the ferromagnetic Curie temperature. Our studies reveal a characteristic length scale for the spatial extent of the donor wavefunctions which remains constant as a function of doping, consistent with recent tunneling studies of doped EuO. Our work sheds light on the nature of the semiconductor-to-metal transition in Eu$_{1-x}$Gd$_{x}$O and should be generally applicable for doped complex oxides.

Details

Database :
arXiv
Journal :
Phys. Rev. B 94, 195102 (2016)
Publication Type :
Report
Accession number :
edsarx.1610.05337
Document Type :
Working Paper
Full Text :
https://doi.org/10.1103/PhysRevB.94.195102