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Polariton Induced Enhanced Emission from an Organic Dye under Strong Coupling Regime

Authors :
Ballarini, Dario
De Giorgi, Milena
Gambino, Salvatore
Lerario, Giovanni
Mazzeo, Marco
Genco, Armando
Accorsi, Gianluca
Giansante, Carlo
Colella, Silvia
D'Agostino, Stefania
Cazzato, Paolo
Sanvitto, Daniele
Gigli, Giuseppe
Source :
Advanced Optical Materials (2014)
Publication Year :
2014

Abstract

Exciton-polaritons in semiconductors are quasi-particles which have recently shown the capability to undergo phase transition into a coherent hybrid state of light and matter. The observation of such quasi-particles in organic microcavities has attracted increasing attention for their characteristic of reaching condensation at room temperature. In this work we demonstrate that the emission properties of organic polaritons do not depend on the overlap between the absorption and emission states of the molecule and that the emission dynamics are modified in the strong coupling regime, showing a significant enhancement of the photoluminescence intensity as compared to the bare dye. This paves the way to the investigation of molecules with large absorption coefficients but poor emission efficiencies for the realization of polariton condensates and organic electrically injected lasers by exploiting strong exciton-photon coupling regimes.

Details

Database :
arXiv
Journal :
Advanced Optical Materials (2014)
Publication Type :
Report
Accession number :
edsarx.1410.5268
Document Type :
Working Paper
Full Text :
https://doi.org/10.1002/adom.201400226