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The magnetic and crystal structures of Sr2IrO4: A neutron diffraction study

Authors :
Ye, Feng
Chi, Songxue
Chakoumakos, Bryan C.
Fernandez-Baca, Jaime A.
Qi, Tongfei
Cao, G.
Source :
Physical Review B 87, 140406(R) (2013)
Publication Year :
2013

Abstract

We report a single-crystal neutron diffraction study of the layered $\rm Sr_2IrO_4$. This work unambiguously determines the magnetic structure of the system and reveals that the spin orientation rigidly tracks the staggered rotation of the $\rm IrO_6$ octahedra in $\rm Sr_2IrO_4$. The long-range antiferromagnetic order has a canted spin configuration with an ordered moment of 0.208(3) $\mu_B$/Ir site within the basal plane; a detailed examination of the spin canting yields 0.202(3) and 0.049(2) $\mu_B$/site for the a axis and the b axis, respectively. It is intriguing that forbidden nuclear reflections of space group $I4_1/acd$ are also observed in a wide temperature range from 4 K to 600 K, which suggests a reduced crystal structure symmetry. This neutron-scattering work provides a direct, well-refined experimental characterization of the magnetic and crystal structures that are crucial to the understanding of the unconventional magnetism exhibited in this unusual magnetic insulator.<br />Comment: the version appeared in PRB

Details

Database :
arXiv
Journal :
Physical Review B 87, 140406(R) (2013)
Publication Type :
Report
Accession number :
edsarx.1302.2890
Document Type :
Working Paper
Full Text :
https://doi.org/10.1103/PhysRevB.87.140406