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Unifying explanation for carrier relaxation anomaly in gapped systems

Authors :
Ono, Shota
Shima, Hiroyuki
Toda, Yasunori
Publication Year :
2012

Abstract

We develop a theory to describe energy relaxation of photo-excited carriers in low-temperature ordered states with band gap opening and formulate carrier relaxation time $\tau$ near and below transition temperature $T_{\mathrm{c}}$ by quantifying contributions from different carrier-phonon scatterings to the relaxation rate. The theory explains anomalous experimental observations of $\tau$ in gapped systems. Transverse acoustic (TA) phonon modes play a crucial role in carrier relaxation; their heat capacity determines $\tau$-divergence near $T_{\mathrm{c}}$. The theory is validated by fitting $\tau$ of fullerene polymers onto a theoretical curve.<br />Comment: 5 pages, 3 figures

Details

Database :
arXiv
Publication Type :
Report
Accession number :
edsarx.1202.2635
Document Type :
Working Paper