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Observation of dose-rate dependence in a Fricke dosimeter irradiated at low dose rates with monoenergetic X-rays

Authors :
O’Leary, Mel
Boscolo, Daria
Breslin, Nicole
Brown, Jeremy M. C.
Dolbnya, Igor P.
Emerson, Chris
Figueira, Catarina
Fox, Oliver J. L.
Grimes, David Robert
Ivosev, Vladimir
Kleppe, Annette K.
McCulloch, Aaron
Pape, Ian
Polin, Chris
Wardlow, Nathan
Currell, Fred J.
Source :
O'Leary, M, Boscolo, D, Breslin, N, Brown, J, Dolbnya, I P, Emerson, C, Figueira, C, Fox, O J L, Crimes, D R, Ivosev, V, Kleppe, A K, McCulloch, A, Pape, I, Polin, C, Wardlow, N & Currell, F 2018, ' Observation of dose-rate dependence in a Fricke dosimeter irradiated at low dose rates with monoenergetic X-rays ', Scientific Reports, vol. 8, 4735, pp. 1-9 . https://doi.org/10.1038/s41598-018-21813-z, Scientific Reports, 8(1), Scientific Reports, Scientific Reports, Vol 8, Iss 1, Pp 1-9 (2018), Scientific reports 8(1), 4735 (2018). doi:10.1038/s41598-018-21813-z, O'Leary, M, Boscolo, D, Breslin, N, Brown, J M C, Dolbnya, I P, Emerson, C, Figueira, C, Fox, O J L, Grimes, D R, Ivosev, V, Kleppe, A K, McCulloch, A, Pape, I, Polin, C, Wardlow, N & Currell, F 2018, ' Observation of dose-rate dependence in a Fricke dosimeter irradiated at low dose rates with monoenergetic X-rays ', Scientific Reports . https://doi.org/10.1038/s41598-018-21813-z
Publication Year :
2018

Abstract

Absolute measurements of the radiolytic yield of Fe3+ in a ferrous sulphate dosimeter formulation (6 mM Fe2+), with a 20 keV x-ray monoenergetic beam, are reported. Dose-rate suppression of the radiolytic yield was observed at dose rates lower than and different in nature to those previously reported with x-rays. We present evidence that this effect is most likely to be due to recombination of free radicals radiolytically produced from water. The method used to make these measurements is also new and it provides radiolytic yields which are directly traceable to the SI standards system. The data presented provides new and exacting tests of radiation chemistry codes.

Details

Language :
English
ISSN :
20452322
Database :
OpenAIRE
Journal :
O'Leary, M, Boscolo, D, Breslin, N, Brown, J, Dolbnya, I P, Emerson, C, Figueira, C, Fox, O J L, Crimes, D R, Ivosev, V, Kleppe, A K, McCulloch, A, Pape, I, Polin, C, Wardlow, N & Currell, F 2018, ' Observation of dose-rate dependence in a Fricke dosimeter irradiated at low dose rates with monoenergetic X-rays ', Scientific Reports, vol. 8, 4735, pp. 1-9 . https://doi.org/10.1038/s41598-018-21813-z, Scientific Reports, 8(1), Scientific Reports, Scientific Reports, Vol 8, Iss 1, Pp 1-9 (2018), Scientific reports 8(1), 4735 (2018). doi:10.1038/s41598-018-21813-z, O'Leary, M, Boscolo, D, Breslin, N, Brown, J M C, Dolbnya, I P, Emerson, C, Figueira, C, Fox, O J L, Grimes, D R, Ivosev, V, Kleppe, A K, McCulloch, A, Pape, I, Polin, C, Wardlow, N & Currell, F 2018, ' Observation of dose-rate dependence in a Fricke dosimeter irradiated at low dose rates with monoenergetic X-rays ', Scientific Reports . https://doi.org/10.1038/s41598-018-21813-z
Accession number :
edsair.pmid.dedup....6447d3a5e1f4b4049e2b7753db0cf5dc