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Vibronic and magnetic excitations in the spin-orbital liquid state of FeSc2S4

Authors :
A, Krimmel
M, Mücksch
V, Tsurkan
M M, Koza
H, Mutka
A, Loidl
Source :
Physical review letters. 94(23)
Publication Year :
2004

Abstract

Inelastic neutron scattering results on the spin-orbital liquid in FeSc2S4 are presented. This sulfospinel reveals strong geometric frustration in the spin and in the orbital sector. In the present experiments the orbital liquid is evidenced by a clear spectroscopic signature of a dynamic Jahn-Teller effect with a vibronic splitting 3Gamma approximately 2 meV in agreement with theoretical estimates. The excitations of the spin liquid reveal strong dispersion and can be characterized as cooperative spin excitations in a supercooled paramagnet with a spin gap of Delta approximately 0.2 meV.

Details

ISSN :
00319007
Volume :
94
Issue :
23
Database :
OpenAIRE
Journal :
Physical review letters
Accession number :
edsair.pmid..........f3f2608d86dd011685ba2070b8a94974