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Layer-Number-Dependent Antiferromagnetic and Ferromagnetic Behavior in MnSb_{2}Te_{4}

Authors :
Zhihao, Zang
Yaozheng, Zhu
Ming, Xi
Shangjie, Tian
Tingting, Wang
Pingfan, Gu
Yuxuan, Peng
Shiqi, Yang
Xiaolong, Xu
Yanping, Li
Bo, Han
Liwei, Liu
Yeliang, Wang
Peng, Gao
Jinbo, Yang
Hechang, Lei
Yuan, Huang
Yu, Ye
Source :
Physical review letters. 128(1)
Publication Year :
2021

Abstract

MnBi_{2}Te_{4}, an intrinsic magnetic topological insulator, has shown layer-number-correlated magnetic and topological phases. More interestingly, in the isostructural material MnSb_{2}Te_{4}, the antiferromagnetic (AFM) and ferromagnetic (FM) states have been both observed in the bulk counterparts, which are also predicted to be topologically nontrivial. Revealing the layer-number-dependent magnetic properties of MnSb_{2}Te_{4} down to a single septuple layer (SL) is of great significance for exploring the topological phenomena. However, this is still elusive. Here, using the polar reflective magnetic circular dichroism spectroscopy, both the A-type AFM and FM behaviors are observed and comprehensively studied in MnSb_{2}Te_{4} down to a single SL limit. In A-type AFM MnSb_{2}Te_{4} flakes, an obvious odd-even layer-number effect is observed. An additional surface spin-flop (SSF) transition occurs in even-SL flakes with the number of layers larger than 2. With the AFM linear-chain model, we identify that the even-SL flakes stabilize in a collinear state between the SSF transition and the spin-flop transition due to their appropriate energy ratio between the magnetic-field-scale anisotropy and interlayer interaction. In FM MnSb_{2}Te_{4} flakes, we observe very different magnetic behaviors with an abrupt spin-flipping transition and very small saturation fields, indicating a weakened interlayer interaction. By revealing the rich magnetic states of few-SL MnSb_{2}Te_{4} on the parameter space of the number of layers, external magnetic field, and temperature, our findings pave the way for further quantum transport studies of few-SL MnSb_{2}Te_{4}.

Details

ISSN :
10797114
Volume :
128
Issue :
1
Database :
OpenAIRE
Journal :
Physical review letters
Accession number :
edsair.pmid..........a16fa422db6df2c1d8474289fcb079f9