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Aerosol chemical composition at Cabauw, the Netherlands as observed in two intensive periods in May 2008 and March 2009

Authors :
Mensah, A.A.
Holzinger, R.
Otjes, R.
Trimborn, A.
Mentel, T.F.
Brink, H. ten
Henzing, B.
Kiendler-Scharr, A.
Source :
Atmospheric Chemistry and Physics Discussions, 10, 12, 4723-4742
Publication Year :
2012

Abstract

Observations of aerosol chemical composition in Cabauw, the Netherlands, are presented for two intensive measurement periods in May 2008 and March 2009. Sub-micron aerosol chemical composition was measured by an Aerodyne Aerosol Mass Spectrometer (AMS) and is compared to observations from aerosol size distribution measurements as well as composition measurements with a Monitor for AeRosol and GAses (MARGA) based instrument and a Thermal-desorption Proton-transfer-reaction Mass-spectrometer (TD-PTR-MS). An overview of the data is presented and the data quality is discussed. In May 2008 enhanced pollution was observed with organics contributing 40% to the PM1 mass. In contrast the observed average mass loading was lower in March 2009 and a dominance of ammonium nitrate (42%) was observed. The semi-volatile nature of ammonium nitrate is evidenced in the diurnal cycles with maximum concentrations observed in the morning hours in May 2008 and little diurnal variation observed in March 2009. Size dependent composition data from AMS measurements are presented and show a dominance of organics in the size range below 200 nm. © 2011 Author(s).

Details

Language :
English
Database :
OpenAIRE
Journal :
Atmospheric Chemistry and Physics Discussions, 10, 12, 4723-4742
Accession number :
edsair.od.....10718..77ca5498fab9debb63eec9b0f948c7ec