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Observation of giant and tunable thermal diffusivity of a Dirac fluid at room temperature

Authors :
Niels C. H. Hesp
Alessandro Principi
Klaas-Jan Tielrooij
Frank H. L. Koppens
Alexander Block
Kenji Watanabe
Aron W. Cummings
Matz Liebel
Takashi Taniguchi
Niek F. van Hulst
Stephan Roche
European Commission
Generalitat de Catalunya
Ministerio de Economía y Competitividad (España)
Source :
Dipòsit Digital de Documents de la UAB, Universitat Autònoma de Barcelona, Nature Nanotechnology, Digital.CSIC. Repositorio Institucional del CSIC, instname
Publication Year :
2021
Publisher :
Springer Science and Business Media LLC, 2021.

Abstract

Conducting materials typically exhibit either diffusive or ballistic charge transport. When electron–electron interactions dominate, a hydrodynamic regime with viscous charge flow emerges1–13. More stringent conditions eventually yield a quantum-critical Dirac-fluid regime, where electronic heat can flow more efficiently than charge14–22. However, observing and controlling the flow of electronic heat in the hydrodynamic regime at room temperature has so far remained elusive. Here we observe heat transport in graphene in the diffusive and hydrodynamic regimes, and report a controllable transition to the Dirac-fluid regime at room temperature, using carrier temperature and carrier density as control knobs. We introduce the technique of spatiotemporal thermoelectric microscopy with femtosecond temporal and nanometre spatial resolution, which allows for tracking electronic heat spreading. In the diffusive regime, we find a thermal diffusivity of roughly 2,000 cm2 s−1, consistent with charge transport. Moreover, within the hydrodynamic time window before momentum relaxation, we observe heat spreading corresponding to a giant diffusivity up to 70,000 cm2 s−1, indicative of a Dirac fluid. Our results offer the possibility of further exploration of these interesting physical phenomena and their potential applications in nanoscale thermal management.<br />Spatiotemporal thermoelectric microscopy enables the observation of electronic heat flow in graphene in diffusive and hydrodynamic regimes at room temperature, as well as a controlled transition from a Fermi liquid to Dirac fluid.

Details

ISSN :
17483395 and 17483387
Volume :
16
Database :
OpenAIRE
Journal :
Nature Nanotechnology
Accession number :
edsair.doi.dedup.....f867d9b75102de13448b4b93fba81572
Full Text :
https://doi.org/10.1038/s41565-021-00957-6