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Synthetic Access to All Four Stereoisomers of Oxetin

Authors :
Thao Anh Minh Nguyen
Régis Guillot
Ahmad F Kassir
Florence Charnay-Pouget
David J. Aitken
Marie-Christine Scherrmann
Thomas Boddaert
Sherif Shaban Ragab
Institut de Chimie Moléculaire et des Matériaux d'Orsay (ICMMO)
Université Paris-Sud - Paris 11 (UP11)-Institut de Chimie du CNRS (INC)-Centre National de la Recherche Scientifique (CNRS)
National Research Center [Caire, Egypte]
Institut de Chimie de Clermont-Ferrand (ICCF)
SIGMA Clermont (SIGMA Clermont)-Institut de Chimie du CNRS (INC)-Université Clermont Auvergne [2017-2020] (UCA [2017-2020])-Centre National de la Recherche Scientifique (CNRS)
Source :
Journal of Organic Chemistry, Journal of Organic Chemistry, 2016, 81 (20), pp.9983-9991. ⟨10.1021/acs.joc.6b01795⟩
Publication Year :
2016
Publisher :
American Chemical Society (ACS), 2016.

Abstract

A short synthesis of all four stereoisomers of 3-amino-2-oxetanecarboxylic acid (oxetin) is described. The oxetane core is built using a Paternò-Büchi photochemical [2 + 2] cycloaddition; from the key intermediates, complementary resolution protocols provide access to enantiomerically pure oxetin and epi-oxetin on gram-scale.

Details

ISSN :
15206904 and 00223263
Volume :
81
Database :
OpenAIRE
Journal :
The Journal of Organic Chemistry
Accession number :
edsair.doi.dedup.....ed2e502bd8b621b6e4f787e503ac30f4
Full Text :
https://doi.org/10.1021/acs.joc.6b01795