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Upward revision of global fossil fuel methane emissions based on isotope database

Authors :
James W. C. White
Owen A. Sherwood
Bruce H. Vaughn
Lori Bruhwiler
Edward J. Dlugokencky
Stefan Schwietzke
Giuseppe Etiope
Victoria A. Arling
S. E. Michel
John B. Miller
Pieter P. Tans
Source :
Nature. 538:88-91
Publication Year :
2016
Publisher :
Springer Science and Business Media LLC, 2016.

Abstract

Revisions in isotopic source signatures reveal that global total fossil fuel methane emissions from industry plus natural geological seepage are much larger than thought. Stefan Schwietzke et al. re-evaluate the global methane budget and the contribution of the fossil fuel industry to methane emissions on the basis of long-term global methane and methane carbon isotope records. They find that total fossil fuel methane emissions (fossil fuel industry plus natural geological methane seepage) are not increasing over time, but are 60–110 per cent greater than was previously thought. They also conclude that methane emissions from natural gas, oil and coal production and their usage are 20–60 per cent greater than inventories and that methane emissions from natural gas as a fraction of production have declined from about 8 per cent to 2 per cent over the past three decades. Methane has the second-largest global radiative forcing impact of anthropogenic greenhouse gases after carbon dioxide, but our understanding of the global atmospheric methane budget is incomplete. The global fossil fuel industry (production and usage of natural gas, oil and coal) is thought to contribute 15 to 22 per cent of methane emissions1,2,3,4,5,6,7,8,9,10 to the total atmospheric methane budget11. However, questions remain regarding methane emission trends as a result of fossil fuel industrial activity and the contribution to total methane emissions of sources from the fossil fuel industry and from natural geological seepage12,13, which are often co-located. Here we re-evaluate the global methane budget and the contribution of the fossil fuel industry to methane emissions based on long-term global methane and methane carbon isotope records. We compile the largest isotopic methane source signature database so far, including fossil fuel, microbial and biomass-burning methane emission sources. We find that total fossil fuel methane emissions (fossil fuel industry plus natural geological seepage) are not increasing over time, but are 60 to 110 per cent greater than current estimates1,2,3,4,5,6,7,8,9,10 owing to large revisions in isotope source signatures. We show that this is consistent with the observed global latitudinal methane gradient. After accounting for natural geological methane seepage12,13, we find that methane emissions from natural gas, oil and coal production and their usage are 20 to 60 per cent greater than inventories1,2. Our findings imply a greater potential for the fossil fuel industry to mitigate anthropogenic climate forcing, but we also find that methane emissions from natural gas as a fraction of production have declined from approximately 8 per cent to approximately 2 per cent over the past three decades.

Details

ISSN :
14764687 and 00280836
Volume :
538
Database :
OpenAIRE
Journal :
Nature
Accession number :
edsair.doi.dedup.....e8522baa890b40984e5f20e2a81988ea
Full Text :
https://doi.org/10.1038/nature19797