Back to Search Start Over

The ice-nucleating activity of African mineral dust in the Caribbean boundary layer

Authors :
Alexander D. Harrison
Daniel O’Sullivan
Michael P. Adams
Grace C. E. Porter
Edmund Blades
Cherise Brathwaite
Rebecca Chewitt-Lucas
Cassandra Gaston
Rachel Hawker
Ovid O. Krüger
Leslie Neve
Mira L. Pöhlker
Christopher Pöhlker
Ulrich Pöschl
Alberto Sanchez-Marroquin
Andrea Sealy
Peter Sealy
Mark D. Tarn
Shanice Whitehall
James B. McQuaid
Kenneth S. Carslaw
Joseph M. Prospero
Benjamin J. Murray
Source :
Atmospheric Chemistry and Physics
Publication Year :
2022

Abstract

African mineral dust is transported many thousands of kilometres from its source regions and, because of its ability to nucleate ice, it plays a major role in cloud glaciation around the globe. The ice-nucleating activity of desert dust is influenced by its mineralogy, which varies substantially between source regions and across particle sizes. However, in models it is often assumed that the activity (expressed as active sites per unit surface area as a function of temperature) of atmospheric mineral dust is the same everywhere on the globe. Here, we find that the ice-nucleating activity of African desert dust sampled in the summertime marine boundary layer of Barbados (July and August, 2017) is substantially lower than parameterizations based on soil from specific locations in the Saharan desert or dust sedimented from dust storms. We conclude that the activity of dust in Barbados’ boundary layer is primarily defined by the low K-feldspar content of the dust, which is around 1 %. We propose that the dust we sampled in the Caribbean was from a region in West Africa (in and around the Sahel in Mauritania and Mali), which has a much lower feldspar content than other African sources across the Sahara and Sahel.

Subjects

Subjects :
Atmospheric Science

Details

Language :
English
ISSN :
16807324
Database :
OpenAIRE
Journal :
Atmospheric Chemistry and Physics
Accession number :
edsair.doi.dedup.....e2b2f23b489a911eeee05af1ecadf488