Magnetic excitations in long-range stripe-ordered Pr2NiO4+δ

We report an inelastic neutron scattering study on the magnetic excitations of ${\mathrm{Pr}}_{2}{\mathrm{NiO}}_{4+\ensuremath{\delta}}$ ($\ensuremath{\delta}\ensuremath{\sim}0.24\ifmmode\pm\else\textpm\fi{}0.01$) at $T=10$ K. Spin stripe ordering becomes pronounced below $\ensuremath{\sim}220$ K with an incommensurability $\ensuremath{\epsilon}\ensuremath{\approx}0.346$, and a strong influence of interstitial oxygen is identified on establishing a long-range spin stripe ordering. Apart from the Goldstone modes emerging from the magnetic satellites (${\mathbf{q}}_{m}$), multiple homologous modes are observed along the spin stripe modulation separated by $\mathrm{\ensuremath{\Delta}}{\mathbf{q}}_{m}\ensuremath{\approx}0.076$ in reciprocal lattice units, which is interpreted by the internal periodicity of the long-range ordered discommensurated spin stripes.