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SPALAX new generation: New process design for a more efficient xenon production system for the CTBT noble gas network

Authors :
Christophe Moulin
Claire Gréau
G. Douysset
T. Taffary
Ludovic Deliere
Sylvain Topin
Alexandre Hovesepian
Gilbert Le Petit
Source :
Journal of Environmental Radioactivity. 149:43-50
Publication Year :
2015
Publisher :
Elsevier BV, 2015.

Abstract

The SPALAX (Système de Prélèvement Automatique en Ligne avec l'Analyse du Xénon) is one of the systems used in the International Monitoring System of the Comprehensive Nuclear Test Ban Treaty (CTBT) to detect radioactive xenon releases following a nuclear explosion. Approximately 10 years after the industrialization of the first system, the CEA has developed the SPALAX New Generation, SPALAX-NG, with the aim of increasing the global sensitivity and reducing the overall size of the system. A major breakthrough has been obtained by improving the sampling stage and the purification/concentration stage. The sampling stage evolution consists of increasing the sampling capacity and improving the gas treatment efficiency across new permeation membranes, leading to an increase in the xenon production capacity by a factor of 2-3. The purification/concentration stage evolution consists of using a new adsorbent Ag@ZSM-5 (or Ag-PZ2-25) with a much larger xenon retention capacity than activated charcoal, enabling a significant reduction in the overall size of this stage. The energy consumption of the system is similar to that of the current SPALAX system. The SPALAX-NG process is able to produce samples of almost 7 cm(3) of xenon every 12 h, making it the most productive xenon process among the IMS systems.

Details

ISSN :
0265931X
Volume :
149
Database :
OpenAIRE
Journal :
Journal of Environmental Radioactivity
Accession number :
edsair.doi.dedup.....d501f87fc3f2a45ee284b94e656225cd