A semi-fluid multi-functional binder for a high-performance silicon anode of lithium-ion batteries

Currently, a variety of binders are developed to inhibit the rapid capacity fading of Si. The Si anodes are mainly enhanced by the chemical bonding effect on the surface of conventional solid-state binders. However, with a huge volume change of silicon, solid binders are easily deactivated. Herein, a semi-fluid binder termed GPC is designed based on a viscoelastic crosslinking network with abundant active sites and self-healing performance. The backbone of the binder network is