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Nucleation and growth bottleneck in the conductivity recovery dynamics of nickelate thin films

Authors :
Jak Chakhalian
Kun Geng
Xiaoran Liu
Elsa Abreu
Richard D. Averitt
Verner Thorsmolle
Jingdi Zhang
Derek Meyers
Publication Year :
2019

Abstract

We investigate THz conductivity dynamics in NdNiO$_3$ and EuNiO$_3$ thin films following a photoinduced thermal quench into the metallic state and reveal a clear contrast between first- and second-order dynamics. While in EuNiO$_3$ the conductivity recovers exponentially, in NdNiO$_3$ the recovery is non-exponential and slower than a simple thermal model. Crucially, it is consistent with first-order dynamics and well-described by a 2d Avrami model, with supercooling leading to metastable phase coexistence. The large transients seen in our films are promising for fast electronic (and magnetic) switching applications.<br />includes supplemental material

Details

Language :
English
Database :
OpenAIRE
Accession number :
edsair.doi.dedup.....bfdd147f77b05fcac14e60a3642492ee