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Tropospheric H2 budget and the response of its soil uptake under the changing environment

Authors :
Philippe Constant
Laurier Poissant
Richard Villemur
Source :
Science of The Total Environment. 407:1809-1823
Publication Year :
2009
Publisher :
Elsevier BV, 2009.

Abstract

Molecular hydrogen (H 2 ) is an indirect greenhouse gas present at the trace level in the atmosphere. So far, the sum of its sources and sinks is close to equilibrium, but its large-scale utilization as an alternative energy carrier would alter its atmospheric burden. The magnitude of the emissions associated with a future H 2 -based economy is difficult to predict and remains a matter of debate. Previous attempts to predict the impact that a future H 2 -based economy would exert on tropospheric chemistry were realized by considering a steady rate of microbial-mediated soil uptake, which is currently responsible of ~ 80% of the tropospheric H 2 losses. Although soil uptake, also known as dry deposition is the most important sink for tropospheric H 2 , microorganisms involved in the activity remain elusive. Given that microbial-mediated H 2 soil uptake is influenced by several environmental factors, global change should exert a significant effect on the activity and then, assuming a steady H 2 soil uptake rate for the future may be mistaken. Here, we present an overview of tropospheric H 2 sources and sinks with an emphasis on microbial-mediated soil uptake process. Future researches are proposed to investigate the influence that global change would exert on H 2 dry deposition and to identify microorganisms involved H 2 soil uptake activity.

Details

ISSN :
00489697
Volume :
407
Database :
OpenAIRE
Journal :
Science of The Total Environment
Accession number :
edsair.doi.dedup.....b616b1dc54b4c820fb156cd6b3b8ba77
Full Text :
https://doi.org/10.1016/j.scitotenv.2008.10.064