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Magic numbers in boson4 he clusters: The auger evaporation mechanism
- Source :
- Molecules, Vol 26, Iss 6244, p 6244 (2021), Molecules, Volume 26, Issue 20
- Publication Year :
- 2021
- Publisher :
- MDPI AG, 2021.
-
Abstract
- The absence of magic numbers in bosonic 4He clusters predicted by all theories since 1984 has been challenged by high-resolution matter-wave diffraction experiments. The observed magic numbers were explained in terms of enhanced growth rates of specific cluster sizes for which an additional excitation level calculated by diffusion Monte Carlo is stabilized. The present theoretical study provides an alternative explanation based on a simple independent particle model of the He clusters. Collisions between cluster atoms in excited states within the cluster lead to selective evaporation via an Auger process. The calculated magic numbers as well as the shape of the number distributions are in quite reasonable agreement with the experiments.
- Subjects :
- Diffraction
Evaporation
Pharmaceutical Science
Auger evaporation
Molecular physics
Article
Analytical Chemistry
Auger
QD241-441
Drug Discovery
Cluster (physics)
Physical and Theoretical Chemistry
Cluster supersonic jet
FIS/03 - FISICA DELLA MATERIA
Boson
Physics
Van der Waals bonds
Van der Waals bond
Organic Chemistry
helium clusters
Helium cluster
cluster supersonic jets
magic numbers
Chemistry (miscellaneous)
Excited state
Molecular Medicine
Diffusion Monte Carlo
Excitation
Magic number
Subjects
Details
- Language :
- English
- Database :
- OpenAIRE
- Journal :
- Molecules, Vol 26, Iss 6244, p 6244 (2021), Molecules, Volume 26, Issue 20
- Accession number :
- edsair.doi.dedup.....b39c04c2c6287c4a79e8f3aba737f83b