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Observation of a universal aggregation mechanism and a possible phase transition in Au sputtered by swift heavy ions
- Source :
- Physical review letters. 100(24)
- Publication Year :
- 2008
-
Abstract
- Two exponents, $\delta$, for size distribution of $n$-atom clusters, $Y(n)\sim n^{-\delta}$, have been found in Au clusters sputtered from embedded Au nanoparticles under swift heavy ion irradiation. For small clusters, below 12.5 nm in size, $\delta$ has been found to be 3/2, which can be rationalized as occurring from a steady state aggregation process with size independent aggregation. For larger clusters, a $\delta$ value of 7/2 is suggested, which might come from a dynamical transition to another steady state where aggregation and evaporation rates are size dependent. In the present case, the observed decay exponents do not support any possibility of a thermodynamic liquid-gas type phase transition taking place, resulting in cluster formation.<br />Comment: 4 pages, 3 figures
- Subjects :
- Physics
Phase transition
Condensed Matter - Materials Science
Statistical Mechanics (cond-mat.stat-mech)
Evaporation
General Physics and Astronomy
Materials Science (cond-mat.mtrl-sci)
FOS: Physical sciences
Charged particle
Ion
Distribution (mathematics)
Swift heavy ion
Transition metal
Cluster (physics)
Atomic physics
Condensed Matter - Statistical Mechanics
Subjects
Details
- ISSN :
- 00319007
- Volume :
- 100
- Issue :
- 24
- Database :
- OpenAIRE
- Journal :
- Physical review letters
- Accession number :
- edsair.doi.dedup.....aa4575d4f32df7e5e92a4177a41040ae