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Observation of a universal aggregation mechanism and a possible phase transition in Au sputtered by swift heavy ions

Authors :
D.P. Mahapatra
Gayatri Sahu
Probodh K. Kuiri
Boby Joseph
Jay Ghatak
D. Kanjilal
H. P. Lenka
Source :
Physical review letters. 100(24)
Publication Year :
2008

Abstract

Two exponents, $\delta$, for size distribution of $n$-atom clusters, $Y(n)\sim n^{-\delta}$, have been found in Au clusters sputtered from embedded Au nanoparticles under swift heavy ion irradiation. For small clusters, below 12.5 nm in size, $\delta$ has been found to be 3/2, which can be rationalized as occurring from a steady state aggregation process with size independent aggregation. For larger clusters, a $\delta$ value of 7/2 is suggested, which might come from a dynamical transition to another steady state where aggregation and evaporation rates are size dependent. In the present case, the observed decay exponents do not support any possibility of a thermodynamic liquid-gas type phase transition taking place, resulting in cluster formation.<br />Comment: 4 pages, 3 figures

Details

ISSN :
00319007
Volume :
100
Issue :
24
Database :
OpenAIRE
Journal :
Physical review letters
Accession number :
edsair.doi.dedup.....aa4575d4f32df7e5e92a4177a41040ae