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Quantum electron liquid and its possible phase transition

Authors :
Sunghun Kim
Joonho Bang
Chan-young Lim
Seung Yong Lee
Jounghoon Hyun
Gyubin Lee
Yeonghoon Lee
Jonathan D. Denlinger
Soonsang Huh
Changyoung Kim
Sang Yong Song
Jungpil Seo
Dinesh Thapa
Seong-Gon Kim
Young Hee Lee
Yeongkwan Kim
Sung Wng Kim
Source :
Nature materials. 21(11)
Publication Year :
2021

Abstract

Purely quantum electron systems exhibit intriguing correlated electronic phases by virtue of quantum fluctuations in addition to electron-electron interactions. To realize such quantum electron systems, a key ingredient is dense electrons decoupled from other degrees of freedom. Here, we report the discovery of a pure quantum electron liquid, which spreads up to ~ 3 {\AA} in the vacuum on the surface of electride crystal. An extremely high electron density and its weak hybridisation with buried atomic orbitals evidence the quantum and pure nature of electrons, that exhibit a polarized liquid phase as demonstrated by our spin-dependent measurement. Further, upon enhancing the electron correlation strength, the dynamics of quantum electrons changes to that of non-Fermi liquid along with an anomalous band deformation, suggestive of a transition to a hexatic liquid crystal phase. Our findings cultivate the frontier of quantum electron systems, and serve as a platform for exploring correlated electronic phases in a pure fashion.<br />Comment: 29 pages, 4 figures, 10 extended data figures

Details

ISSN :
14764660
Volume :
21
Issue :
11
Database :
OpenAIRE
Journal :
Nature materials
Accession number :
edsair.doi.dedup.....a59d30c0d3eb184e84dd884af3bd1789