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Finite-size effects in single chain magnets: an experimental and theoretical study

Authors :
Dante Gatteschi
Alessandro Vindigni
Maria Gloria Pini
Miguel A. Novak
Angelo Rettori
Roberta Sessoli
M. Fedi
Lapo Bogani
M. Massi
Andrea Caneschi
Source :
Physical review letters, 92 (2004): 207274. doi:10.1103/PhysRevLett.92.207204, info:cnr-pdr/source/autori:L. Bogani (1); A. Caneschi (1); M. Fedi 82); D. Gatteschi (1); M. Massi (2); M. A. Novak (3); M. G. Pini (4); A. Rettori (5); R. Sessoli (1); A. Vindigni (5)/titolo:Finite-Size Effects in Single Chain Magnets: An Experimental and Theoretical Study/doi:10.1103%2FPhysRevLett.92.207204/rivista:Physical review letters (Print)/anno:2004/pagina_da:207274/pagina_a:/intervallo_pagine:207274/volume:92
Publication Year :
2003

Abstract

The problem of finite size effects in s=1/2 Ising systems showing slow dynamics of the magnetization is investigated introducing diamagnetic impurities in a Co$^{2+}$-radical chain. The static magnetic properties have been measured and analyzed considering the peculiarities induced by the ferrimagnetic character of the compound. The dynamic susceptibility shows that an Arrhenius law is observed with the same energy barrier for the pure and the doped compounds while the prefactor decreases, as theoretically predicted. Multiple spins reversal has also been investigated.<br />4 pages, 5 figures. Physical Review Letters, accepted for publication

Details

ISSN :
00319007
Volume :
92
Issue :
20
Database :
OpenAIRE
Journal :
Physical review letters
Accession number :
edsair.doi.dedup.....9e5e59ec8067f0bc09650dd866143ff5
Full Text :
https://doi.org/10.1103/PhysRevLett.92.207204