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Coherent and incoherent bands in La and Rh doped Sr$_3$ Ir$_2$ O$_7$

Authors :
Brouet, V.
Serrier-Garcia, L.
Louat, A.
Fruchter, L.
Bertran, F.
Fevre, P. Le
Rault, J.
Forget, A
Colson, D.
Laboratoire de Physique des Solides (LPS)
Centre National de la Recherche Scientifique (CNRS)-Université Paris-Sud - Paris 11 (UP11)
Synchrotron SOLEIL (SSOLEIL)
Centre National de la Recherche Scientifique (CNRS)
Service de physique de l'état condensé (SPEC - UMR3680)
Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)
ANR-15-CE30-0009,SOCRATE,Nouveaux états électroniques corrélés émergeant d'un couplage spin-orbite fort : le cas des iridates(2015)
ANR-11-IDEX-0003,IPS,Idex Paris-Saclay(2011)
Université Paris-Sud - Paris 11 (UP11)-Centre National de la Recherche Scientifique (CNRS)
Source :
Physical Review B: Condensed Matter and Materials Physics (1998-2015), Physical Review B: Condensed Matter and Materials Physics (1998-2015), American Physical Society, 2018, 98, pp.235101. ⟨10.1103/PhysRevB.98.235101⟩, Physical Review B: Condensed Matter and Materials Physics (1998-2015), 2018, 98, pp.235101. ⟨10.1103/PhysRevB.98.235101⟩
Publication Year :
2018
Publisher :
HAL CCSD, 2018.

Abstract

International audience; In Sr$_2$ IrO$_4$ and Sr$_3$ Ir$_2$ O$_7$ , correlations, magnetism, and spin-orbit coupling compete on similar energy scales, creating a new context to study metal-insulator transitions (MIT). We use here angle-resolved photoemission to investigate the MIT as a function of hole and electron doping in Sr$_3$ Ir$_2$ O$_7$ , obtained respectively by Ir/Rh and Sr/La substitutions. We show that there is a clear reduction as a function of doping of the gap between a lower and upper band on both sides of the Fermi level, from 0.2 to 0.05 eV. Although these two bands have a counterpart in band structure calculations, they are characterized by a very different degree of coherence. The upper band exhibits clear quasiparticle peaks, while the lower band is very broad and loses weight as a function of doping. Moreover, their ARPES spectral weights obey different periodicities, reinforcing the idea of their different nature. We argue that a very similar situation occurs in Sr$_2$ IrO$_4$ and conclude that the physics of the two families is essentially the same.

Details

Language :
English
ISSN :
10980121 and 1550235X
Database :
OpenAIRE
Journal :
Physical Review B: Condensed Matter and Materials Physics (1998-2015), Physical Review B: Condensed Matter and Materials Physics (1998-2015), American Physical Society, 2018, 98, pp.235101. ⟨10.1103/PhysRevB.98.235101⟩, Physical Review B: Condensed Matter and Materials Physics (1998-2015), 2018, 98, pp.235101. ⟨10.1103/PhysRevB.98.235101⟩
Accession number :
edsair.doi.dedup.....926edca2817812d9c8d9afe22582ae1b