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Publisher Correction: Carrier lifetime enhancement in halide perovskite via remote epitaxy

Authors :
Yuan Ma
Jian Shi
Daniel Gall
Jing Feng
Baiwei Wang
Zhizhong Chen
Esther Wertz
Xin Sun
Yuwei Guo
Lifu Zhang
Humberto Terrones
Min Chen
Yunfeng Shi
Yuanyuan Zhou
Lei Jin
Lei Gao
Zhiwei Ma
Yang Hu
Nitin P. Padture
Jie Jiang
Kory Beach
Toh-Ming Lu
Fengshan Zheng
Xinchun Chen
Source :
Nature Communications, Vol 10, Iss 1, Pp 1-1 (2019), Nature Communications
Publication Year :
2019
Publisher :
Nature Portfolio, 2019.

Abstract

Crystallographic dislocation has been well-known to be one of the major causes responsible for the unfavorable carrier dynamics in conventional semiconductor devices. Halide perovskite has exhibited promising applications in optoelectronic devices. However, how dislocation impacts its carrier dynamics in the 'defects-tolerant' halide perovskite is largely unknown. Here, via a remote epitaxy approach using polar substrates coated with graphene, we synthesize epitaxial halide perovskite with controlled dislocation density. First-principle calculations and molecular-dynamics simulations reveal weak film-substrate interaction and low density dislocation mechanism in remote epitaxy, respectively. High-resolution transmission electron microscopy, high-resolution atomic force microscopy and Cs-corrected scanning transmission electron microscopy unveil the lattice/atomic and dislocation structure of the remote epitaxial film. The controlling of dislocation density enables the unveiling of the dislocation-carrier dynamic relation in halide perovskite. The study provides an avenue to develop free-standing halide perovskite film with low dislocation density and improved carried dynamics.

Details

Language :
English
ISSN :
20411723
Volume :
10
Issue :
1
Database :
OpenAIRE
Journal :
Nature Communications
Accession number :
edsair.doi.dedup.....8cf9aa948477b87f8c16a82be84b430f