Highly tunable multiple narrow emissions of dyed dielectric-metal core-shell resonators: towards efficient fluorescent labels

We report a potential efficient fluorescent label based on the dyed dielectric-metal core–shell resonators (DMCSRs). By utilizing the near-field coupling between the dyes and the multipolar sharp cavity plasmon resonances, the dyed DMCSRs with diameter of 1.02 μm are demonstrated to be capable of supporting multiple spontaneous emission peaks with the linewidths as narrow as ~ 10 nm in visible range, and these reshaped fluorescent emissions are insensitive to the surrounding dielectric environment. Furthermore, these multiple narrow emission peaks show a precise tunability on the spectrum by simply separating a nanometric dielectric layer between the dielectric core and the metallic shell, which may provide an attractive spectral multiplexing strategy in the fields of cell biology and medical sciences.