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A structure–dynamics relationship in ratcheted colloids: resonance melting, dislocations, and defect clusters

Authors :
Debasish Chaudhuri
Dipanjan Chakraborty
Shubhendu Shekhar Khali
Source :
Soft Matter. 16:2552-2564
Publication Year :
2020
Publisher :
Royal Society of Chemistry (RSC), 2020.

Abstract

We consider a two dimensional colloidal dispersion of soft-core particles driven by a one dimensional stochastic flashing ratchet that induces a time averaged directed particle current through the system. It undergoes a non-equilibrium melting transition as the directed current approaches a maximum associated with a resonance of the ratcheting frequency with the relaxation frequency of the system. We use extensive molecular dynamics simulations to present a detailed phase diagram in the ratcheting rate-mean density plane. With the help of numerically calculated structure factor, solid and hexatic order parameters, and pair correlation functions, we show that the non-equilibrium melting is a continuous transition from a quasi-long ranged ordered solid to a hexatic phase. The transition is mediated by the unbinding of dislocations, and formation of compact and string-like defect clusters.<br />Comment: 12 pages, 14 figures

Details

ISSN :
17446848 and 1744683X
Volume :
16
Database :
OpenAIRE
Journal :
Soft Matter
Accession number :
edsair.doi.dedup.....644434ac0bfa3ef84604b0452b20e75c
Full Text :
https://doi.org/10.1039/c9sm02238d