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Coupling Space-Resolved Dynamic Light Scattering and Rheometry to Investigate Heterogeneous Flow and Nonaffine Dynamics in Glassy and Jammed Soft Matter
- Source :
- Physical Review Applied, Physical Review Applied, American Physical Society, 2019, 11 (3), pp.034073. ⟨10.1103/PhysRevApplied.11.034073⟩
- Publication Year :
- 2019
- Publisher :
- American Physical Society (APS), 2019.
-
Abstract
- International audience; We present a new light scattering setup coupled to a commercial rheometer operated in the plate-plate geometry. The apparatus allows the microscopic dynamics to be measured, discriminating between the contribution due to the affine deformation and additional mechanisms, such as plasticity. Light backscattered by the sample is collected using an imaging optical layout, thereby allowing the average flow velocity and the microscopic dynamics to be probed with both spatial and temporal resolution. We successfully test the setup by measuring the Brownian diffusion and flow velocity of diluted colloidal suspensions, both at rest and under shear. The potentiality of the apparatus are explored in the startup shear of a biogel. For small shear deformations, $\gamma \le 2\%$, the rheological response of the gel is linear. However, striking deviations from affine flow are seen from the very onset of deformation, due to temporally and spatially heterogeneous rearrangements bearing intriguing similarities with a stick-slip process.
- Subjects :
- Materials science
Rheometry
Rheometer
General Physics and Astronomy
02 engineering and technology
Mechanics
Plasticity
021001 nanoscience & nanotechnology
01 natural sciences
Light scattering
Condensed Matter::Soft Condensed Matter
Physics::Fluid Dynamics
Flow velocity
Dynamic light scattering
Rheology
Temporal resolution
0103 physical sciences
010306 general physics
0210 nano-technology
[PHYS.COND.CM-SCM]Physics [physics]/Condensed Matter [cond-mat]/Soft Condensed Matter [cond-mat.soft]
Subjects
Details
- ISSN :
- 23317019
- Volume :
- 11
- Database :
- OpenAIRE
- Journal :
- Physical Review Applied
- Accession number :
- edsair.doi.dedup.....49e317a12ef1452b00b7ccaafdcf983e
- Full Text :
- https://doi.org/10.1103/physrevapplied.11.034073