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Effect of non-thermal plasma in the activation and regeneration of 13X zeolite for enhanced VOC elimination by cycled storage and discharge process

Authors :
Savita Kaliya Perumal Veerapandian
Nathalie De Geyter
Jean-Marc Giraudon
Jean-Charles Morin
Parinaz Saadat Esbah Tabaei
Guy De Weireld
Andreas Laemont
Karen Leus
Pascal Van Der Voort
Jean-François Lamonier
Rino Morent
Universiteit Gent = Ghent University (UGENT)
Department of Applied physics [Ghent]
Unité de Catalyse et Chimie du Solide - UMR 8181 (UCCS)
Université d'Artois (UA)-Centrale Lille-Institut de Chimie du CNRS (INC)-Université de Lille-Centre National de la Recherche Scientifique (CNRS)
Université de Mons (UMons)
Université de Lille
CNRS
Centrale Lille
ENSCL
Univ. Artois
Universiteit Gent = Ghent University [UGENT]
3209|||Unité de Catalyse et Chimie du Solide - UMR 8181 [UCCS]
Université de Mons [UMons]
Unité de Catalyse et Chimie du Solide (UCCS) - UMR 8181
Source :
Journal of Cleaner Production, Journal of Cleaner Production, 2022, 364 (132687), ⟨10.1016/j.jclepro.2022.132687⟩
Publication Year :
2022
Publisher :
HAL CCSD, 2022.

Abstract

International audience; A non-thermal plasma (NTP) discharge is used in this study for the activation and regeneration of MS-13X pellets packed in a MS-13X & glass beads packed bed dielectric barrier discharge (DBD) reactor. NTP activation (in-situ) of MS-13X efficiently removes the adsorbed carbonaceous compounds and moisture resulting in an improved VOC adsorption. In addition, NTP exposure is used for the regeneration of the used MS-13X for cycled storage and discharge (CSD) removal of VOC from air. The amount of adsorbed toluene, products formed and the surface and bulk properties of the regenerated used MS-13X shows complete regeneration of used MS-13X. Finally, the stability of MS-13X during 10 cycles of CSD shows no degradation in performance. Thus, NTP exposure is proven to be successful for both the activation and regeneration of MS-13X pellets used for cyclic CSD process.

Details

Language :
English
ISSN :
09596526
Database :
OpenAIRE
Journal :
Journal of Cleaner Production, Journal of Cleaner Production, 2022, 364 (132687), ⟨10.1016/j.jclepro.2022.132687⟩
Accession number :
edsair.doi.dedup.....4864ffd1323bab7c1a59b66380308cc3
Full Text :
https://doi.org/10.1016/j.jclepro.2022.132687⟩