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Production of 117mSn with high specific activity by cyclotron

Authors :
Zoltan Szucs
Grigory K. Vostokin
V.N. Shvetsov
G. Ya. Starodub
S. N. Dmitriev
O. D. Maslov
M. V. Gustova
Jan Rijn Zeevaart
D. Jansen
Source :
Applied Radiation and Isotopes. 69:965-968
Publication Year :
2011
Publisher :
Elsevier BV, 2011.

Abstract

A method to produce (117m)Sn radionuclide using accelerator production route is described. A new method is proposed to separate the (117m)Sn. Specific activities and thick target yield for (116)Cd(α,3n)(117m)Sn reaction at E(α)=35MeV bombarding energy were determined. The estimated production yield of (117m)Sn was 37.5kBq/μAh for 13.16 mg/cm(2) natural cadmium-oxide target and 410 kBq/μAh for 11.07 mg/cm(2) highly enriched (95%) (116)CdO target. The method developed for separation of (117m)Sn from Cd using anion-exchange resin (Dowex -1×8, fluorine form, 400 mesh) can achieve 98% radiochemical yield of (117m)Sn with more than 99% radionuclidic purity. The estimated specific activity is 2.4 GBq/mg that can be reached with the used irradiation conditions.

Details

ISSN :
09698043
Volume :
69
Database :
OpenAIRE
Journal :
Applied Radiation and Isotopes
Accession number :
edsair.doi.dedup.....3ef2ced26dfc24e6dc7a3dcc6ef3622a
Full Text :
https://doi.org/10.1016/j.apradiso.2011.02.031