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Design and performance of an automated chemical extraction bench for the preparation of 10Be and 26Al targets to be analyzed by accelerator mass spectrometry

Authors :
Valery Guillou
Laëtitia Léanni
Georges Aumaître
Régis Braucher
Karim Keddadouche
Mélanie Baroni
Didier Bourlès
Centre européen de recherche et d'enseignement des géosciences de l'environnement (CEREGE)
Institut de Recherche pour le Développement (IRD)-Institut National de la Recherche Agronomique (INRA)-Aix Marseille Université (AMU)-Collège de France (CdF (institution))-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)
Aix Marseille Université (AMU)-Institut national des sciences de l'Univers (INSU - CNRS)-Collège de France (CdF (institution))-Institut de Recherche pour le Développement (IRD)-Centre National de la Recherche Scientifique (CNRS)-Institut National de la Recherche Agronomique (INRA)
Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Collège de France (CdF)-Institut national des sciences de l'Univers (INSU - CNRS)-Aix Marseille Université (AMU)-Institut National de la Recherche Agronomique (INRA)
Source :
Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, 2019, 456, pp.230-235. ⟨10.1016/j.nimb.2019.04.002⟩, Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Elsevier, 2019, 456, pp.230-235. ⟨10.1016/j.nimb.2019.04.002⟩, Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Elsevier, 2019, ⟨10.1016/j.nimb.2019.04.002⟩
Publication Year :
2019
Publisher :
HAL CCSD, 2019.

Abstract

International audience; The growing number of studies based on data provided by the accelerator mass spectrometry (AMS) technique from increasingly diverse matrices implies that developing very effective and reproducible sample processing techniques is crucial to meet the demand generated. After being dissolved, the isolation of the cosmogenic nuclide to be measured and its chemical purification imply complex processes throughout successive stages The presented automatic system was designed to perform the final steps of the Be-10 and Al-26 chemical extraction protocol from natural matrices (sediments, pure mineral phases, ...), previously purified, decontaminated and dissolved in the case of in situ-produced cosmogenic nuclides, or leached or dissolved in the case of meteoric cosmogenic nuclides. Driven by Labview software, the developed automatic system, in addition to freeing the operator from tedious tasks, allows reproducibly processing simultaneously up to eight samples of different volumes in roughly 40 min. This article presents the design of the automated extraction bench and its performance based on the recovery efficiency of the stable element and the reproducibility of the measurements of the cosmogenic nuclide concentrations by AMS.

Details

Language :
English
ISSN :
0168583X
Database :
OpenAIRE
Journal :
Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, 2019, 456, pp.230-235. ⟨10.1016/j.nimb.2019.04.002⟩, Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Elsevier, 2019, 456, pp.230-235. ⟨10.1016/j.nimb.2019.04.002⟩, Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Elsevier, 2019, ⟨10.1016/j.nimb.2019.04.002⟩
Accession number :
edsair.doi.dedup.....3dbce6af337fa95f13bdda060eba4c8a
Full Text :
https://doi.org/10.1016/j.nimb.2019.04.002⟩