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Many-body interaction effects on the low-k structure of liquid Kr

Authors :
Renato Magli
Luciano Reatto
G. Casanova
M. Tau
Eleonora Guarini
Fabrizio Barocchi
Source :
Physical review. E, Statistical, nonlinear, and soft matter physics. 63(5 Pt 1)
Publication Year :
2000

Abstract

Neutron diffraction measurements and theoretical calculations of the structure factor $S(k)$ of liquid Kr are extended to small k values $(kl4 {\mathrm{nm}}^{\ensuremath{-}1}).$ The results show that many-body interaction contributions have an increasing effect on $S(k)$ as $\stackrel{\ensuremath{\rightarrow}}{k}0,$ reaching at least 40% of the measured intensity. Both the phase diagram and the low-$k$ structural data of dense Kr turn out to be closely reproduced by the hierarchical reference theory if additional many-body forces are taken into account by an augmented strength of the Axilrod-Teller triple-dipole potential. The experimental density derivative of $S(k)$ is also used for a very sensitive test of the theories and interaction models considered here.

Details

ISSN :
15393755
Volume :
63
Issue :
5 Pt 1
Database :
OpenAIRE
Journal :
Physical review. E, Statistical, nonlinear, and soft matter physics
Accession number :
edsair.doi.dedup.....3bf15437ae7380de2077ca20d6cc9260