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Collective dynamics of liquid deuterium: Neutron scattering and approximate quantum simulation methods

Authors :
Alessandro Cunsolo
Renato Magli
Ubaldo Bafile
Milva Celli
Fabrizio Barocchi
Eleonora Guarini
Martin Neumann
Ferdinando Formisano
Daniele Colognesi
A. Laloni
Alessio De Francesco
Source :
Physical Review B 104 (2021). doi:10.1103/PhysRevB.104.174204, info:cnr-pdr/source/autori:Eleonora Guarini, Fabrizio Barocchi, Alessio De Francesco, Ferdinando Formisano, Alessio Laloni, Ubaldo Bafile, Milva Celli, Daniele Colognesi, Renato Magli, Alessandro Cunsolo, Martin Neumann./titolo:Collective dynamics of liquid deuterium: Neutron scattering and approximate quantum simulation methods/doi:10.1103%2FPhysRevB.104.174204/rivista:Physical Review B/anno:2021/pagina_da:/pagina_a:/intervallo_pagine:/volume:104
Publication Year :
2021
Publisher :
American Physical Society (APS), 2021.

Abstract

We present an experimental and simulation study of the collective dynamics of liquid D2 in the range of exchanged wave vectors 3< Q< 14 nm-1. Neutron Brillouin scattering results for the center-of-mass dynamic structure factor of this moderately quantum fluid are compared, on an absolute scale, with those obtained by three different quantum simulation methods such as ring polymer molecular dynamics and two versions of the Feynman-Kleinert approach. The experimental data can be well described by dynamical models typically used for liquids. Some discrepancies show up both among simulations, and between simulations and experimental data. Such discrepancies are found to mainly concern the damping of the propagating sound modes.

Details

ISSN :
24699969 and 24699950
Volume :
104
Database :
OpenAIRE
Journal :
Physical Review B
Accession number :
edsair.doi.dedup.....34f37e48c11870b1420bd14c9df969e9