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Spin Polarization, Electron–Phonon Coupling, and Zero-Phonon Line of the NV Center in 3C-SiC
- Source :
- Nano Letters, Nano Letters, American Chemical Society, 2021, 21 (19), pp.8119-8125. ⟨10.1021/acs.nanolett.1c02564⟩
- Publication Year :
- 2021
- Publisher :
- American Chemical Society (ACS), 2021.
-
Abstract
- International audience; The nitrogen-vacancy (NV) center in 3C-SiC, the analog of the NV center in diamond, has recently emerged as a solid-state qubit with competitive properties and significant technological advantages. Combining first-principles calculations and magnetic resonance spectroscopy we provide thorough insight in its magneto-optical properties. By applying resonantly excited electron paramagnetic resonance spectroscopy, we identified the zero-phonon absorption line of the 3 A 2 → 3 E transition at 1289 nm (within the telecom Oband) and measured its phonon sideband, the analysis of which reveals a Huang-Rhys factor of S = 2.85 and a Debye-Waller factor of 5.8 %. The low temperature spin-lattice relaxation time was found to be exceptionally long (T 1 = 17 s at 4 K). All these properties make NV in 3C-SiC a strong competitor for qubit application. In addition, the strong variation of the zero-field splitting in the range of 4K to 380K allows its application for nanoscale thermal sensing.
- Subjects :
- Phonon
Bioengineering
02 engineering and technology
01 natural sciences
7. Clean energy
Spectral line
Paramagnetism
silicon carbide
0103 physical sciences
resonant excitation
[CHIM]Chemical Sciences
General Materials Science
010306 general physics
Spectroscopy
Physics
Condensed matter physics
Spin polarization
Mechanical Engineering
Resonance
General Chemistry
spin polarization
021001 nanoscience & nanotechnology
Condensed Matter Physics
nitrogen-vacancy color centers
Qubit
Excited state
electron-phonon coupling
0210 nano-technology
Subjects
Details
- ISSN :
- 15306992 and 15306984
- Volume :
- 21
- Database :
- OpenAIRE
- Journal :
- Nano Letters
- Accession number :
- edsair.doi.dedup.....34cd396da55bebd2ad2d75e9744ac985