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Pericyclic reaction benchmarks: hierarchical computations targeting CCSDT(Q)/CBS and analysis of DFT performance

Authors :
Pascal Vermeeren
Marco Dalla Tiezza
Mark E. Wolf
Mitchell E. Lahm
Wesley D. Allen
Henry F. Schaefer
Trevor A. Hamlin
F. Matthias Bickelhaupt
Source :
PCCP Physical Chemistry Chemical Physics, 24, 18028-18042, PCCP Physical Chemistry Chemical Physics, 24, 30, pp. 18028-18042
Publication Year :
2022

Abstract

A hierarchical ab initio benchmark up to CCSDT(Q)/CBS in combination with a DFT performance study reveals meta-hybrid M06-2X functional as the best performing functional for accurately describing pericyclic reactions.

Details

ISSN :
14639076
Database :
OpenAIRE
Journal :
PCCP Physical Chemistry Chemical Physics, 24, 18028-18042, PCCP Physical Chemistry Chemical Physics, 24, 30, pp. 18028-18042
Accession number :
edsair.doi.dedup.....313a573d5e4d3b5099217f8995f36cf3