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Experimental and theoretical study of electronic correlations in carbon nanotubes and graphite from Auger spectroscopy

Authors :
S Ugenti
M. A. El Khakani
F. Rosei
M. De Crescenzi
Enrico Perfetto
Paola Castrucci
Manuela Scarselli
Michele Cini
Publication Year :
2008
Publisher :
IOP Publishing Limited, 2008.

Abstract

We give a quantitative estimate of the screened on-site Coulomb repulsion U in carbon nanotubes and graphite. This is obtained by measuring the Auger spectrum of these materials and performing a theoretical study based on the Green's function method proposed by Cini[Solid. St. Comm. 24, 681 (1977)]. The experimental lineshape is very well reproduced by the theory, where only one fit parameter is employed. This allows to extract the value of the screened on-site repulsion between 2p states, which results U = 4.6 eV for nanotubes and U = 2.1 eV for graphite.

Details

Language :
English
Database :
OpenAIRE
Accession number :
edsair.doi.dedup.....1df6b720373861671fe87edd92ac929d