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Unconventional Biradical Character of Titanium Enolates

Authors :
Pedro Romea
Josep M. Anglada
Joaquim Nebot
I. de P. R. Moreira
Fèlix Urpí
Joan G. Solsona
Josep Maria Bofill
Source :
Journal of the American Chemical Society. 130:3242-3243
Publication Year :
2008
Publisher :
American Chemical Society (ACS), 2008.

Abstract

Experimental and theoretical studies evidence an unconventional biradical character for the titanium enolates derived from α-alkoxy ketones and TiCl4. EPR experiments and ab initio calculations suggest that these titanium enolates have an open shell electronic ground state.

Details

ISSN :
15205126 and 00027863
Volume :
130
Database :
OpenAIRE
Journal :
Journal of the American Chemical Society
Accession number :
edsair.doi.dedup.....0376a28670edba217e521b5faffbb6f2