Electronic processes occurring during ultrafast demagnetization of cobalt triggered by x-ray photons tuned to the Co L 3 resonance

Physical review / B 107(9), 094402 (2023). doi:10.1103/PhysRevB.107.094402
Magnetization dynamics triggered by ultrashort laser pulses has been attracting significant attention, with a strong focus on the dynamics excited by visible/near-infrared pulses. Only recently has a strong magnetic response in solid materials induced by intense x-ray pulses from free-electron lasers been observed. The exact mechanisms that trigger the x-ray-induced demagnetization are not yet fully understood. They are the subject of ongoing experimental and theoretical investigations. Here, we present a theoretical analysis of electronic processes occurring during demagnetization of a Co multilayer system irradiated by x-ray pulses tuned to the $L_3$ absorption edge of cobalt. We show that, like in the case of x-ray-induced demagnetization at the $M$ edge of Co, electronic processes play a predominant role in the demagnetization until the pulse fluence does not exceed the structural damage threshold. The impact of electronic processes can explain reasonably well the available experimental data, without a need to introduce the mechanism of stimulated elastic forward scattering.
Published by Inst., Woodbury, NY