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Evidence of local structural order and spin-lattice coupling in the frustrated pyrochloreY2Ru2O7
- Source :
- Physical Review B. 91
- Publication Year :
- 2015
- Publisher :
- American Physical Society (APS), 2015.
-
Abstract
- We present an extended x-ray absorption fine structure study of the pyrochlore ${\mathrm{Y}}_{2}{\mathrm{Ru}}_{2}{\mathrm{O}}_{7}$ (8--298 K). We find evidence, on a local scale, of a significant magnetoelastic coupling at the N\'eel temperature ${T}_{\mathrm{N}}\ensuremath{\sim}77\phantom{\rule{0.28em}{0ex}}\mathrm{K}$ pointed out by a huge Debye-Waller ${\ensuremath{\sigma}}^{2}$ factor deviation from a correlated temperature dependent Debye-like local order behavior plus a temperature independent static contribution. Moreover, we notice the occurrence of a potential local order-disorder structural phase transition at ${T}^{*}=150$ K. This anomalous behavior is consistent with the pyrochlore's predisposition towards structural disorder and with a strong spin-phonon correlation. Remarkably the low-temperature order competes with the tendency of magnetic frustration to induce a less symmetric local structure.
- Subjects :
- Physics
Condensed matter physics
Temperature independent
Pyrochlore
Order (ring theory)
Anomalous behavior
engineering.material
Condensed Matter Physics
Coupling (probability)
Electronic, Optical and Magnetic Materials
Spin lattice
Magnetic frustration
engineering
Condensed Matter::Strongly Correlated Electrons
Absorption (logic)
Subjects
Details
- ISSN :
- 1550235X and 10980121
- Volume :
- 91
- Database :
- OpenAIRE
- Journal :
- Physical Review B
- Accession number :
- edsair.doi...........aa3f2e23c99b314acc360ea2206cfee6