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182Hf, a new isotope for AMS

Authors :
Christof Vockenhuber
Alfred Priller
Walter Kutschera
Max Bichler
Peter Steier
Stephan R. Winkler
Robin Golser
Source :
Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms. :823-828
Publication Year :
2004
Publisher :
Elsevier BV, 2004.

Abstract

The neutron-rich isotope 182Hf with its half-life of 9 ± 2 million years was alive in the early solar system and has been used to study the early development of the Earth and the Moon through isotopic anomalies of its stable decay product 182W. In addition, 182Hf may also complement a few other radionuclides in the million-year half-life range to trace relatively recent stellar events with high neutron fluxes in the vicinity of the Earth. This may be accomplished by finding measurable traces of live 182Hf in suitable terrestrial archives. With accelerator mass spectrometry (AMS) it should be possible to detect minute amounts of 182Hf. We will show that the main interference for the detection, the stable isobar 182W, can be significantly reduced by using HfF5− ions. The AMS detection method of 182Hf and first results from Hf control rods of a recently retired research reactor are presented, which encourage us to search for naturally produced traces of 182Hf on Earth.

Details

ISSN :
0168583X
Database :
OpenAIRE
Journal :
Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms
Accession number :
edsair.doi...........aa3c7abe3095e0e0122804e9dbe46667
Full Text :
https://doi.org/10.1016/j.nimb.2004.04.152