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Scanning Tunneling Microscopy-Induced Light Emission and I(V) Study of Optical Near-Field Properties of Single Plasmonic Nanoantennas

Authors :
Anton Samusev
Alexey M. Mozharov
V. A. Shkoldin
D. V. Lebedev
Dmitry V. Permyakov
Lilia N Dvoretckaia
Andrey Bogdanov
Ivan Mukhin
Alexander Golubok
Source :
The Journal of Physical Chemistry Letters. 12:501-507
Publication Year :
2020
Publisher :
American Chemical Society (ACS), 2020.

Abstract

Electrically driven plasmonic nanoantennas can be integrated as a local source of the optical signal of advanced photonic schemes for on-chip data processing. The inelastic electron tunneling provides the photon generation or launch of surface plasmon waves. This process can be enhanced by the local density of optical states of nanoantennas. In this paper, we used scanning tunnel microscopy-induced light emission to probe the local optoelectronic properties of single gold nanodiscs. The electromagnetic field distribution in the vicinity of plasmonic structures was investigated with high spatial resolution. The obtained photon maps reveal the nonuniform distribution of electromagnetic near-fields, which is consistent with nanoantenna optical modes. Also, the analysis of derived I(V) curves showed a direct correlation between the nanoantenna optical states and the appearance of features on current-voltage characteristics.

Details

ISSN :
19487185
Volume :
12
Database :
OpenAIRE
Journal :
The Journal of Physical Chemistry Letters
Accession number :
edsair.doi...........93456d0e6cf973aeacbaca00f69cbd21
Full Text :
https://doi.org/10.1021/acs.jpclett.0c03039