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Ultrafast resonant soft x-ray diffraction dynamics of the charge density wave inTbTe3

Authors :
Oleg Krupin
Wei-Sheng Lee
Joshua J. Turner
T. P. Devereaux
Y.-D. Chuang
Mariano Trigo
William F. Schlotter
Alexander F. Kemper
Donghui Lu
David A. Reis
Ph. Hering
Zahid Hussain
T. Benson
Robert G. Moore
Jiun-Haw Chu
Peter Denes
Dionisio Doering
Ian R. Fisher
Ming Yi
Zhi-Xun Shen
P. S. Kirchman
G. Hays
L. Patthey
Source :
Physical Review B. 93
Publication Year :
2016
Publisher :
American Physical Society (APS), 2016.

Abstract

Understanding the emergence of collective behavior in correlated electron systems remains at the forefront of modern condensed matter physics. Disentangling the degrees of freedom responsible for collective behavior can lead to insights into the microscopic origins of emergent properties and phase transitions. Utilizing an optical pump, resonant soft x-ray diffraction probe we are able to track, in real time, the dynamics of the charge density wave (CDW) in ${\mathrm{TbTe}}_{3}$, a model system that violates traditional views of a Fermi surface nested CDW. We observe coherent oscillations corresponding to the CDW amplitude mode at $2.4$ THz and a coherent optical phonon mode at $\ensuremath{\sim}1.7\phantom{\rule{0.16em}{0ex}}\mathrm{THz}$. We show how such observations reveal the anisotropic energy optimization between in-plane Te charge density modulations and the three-dimensional lattice coupling.

Details

ISSN :
24699969 and 24699950
Volume :
93
Database :
OpenAIRE
Journal :
Physical Review B
Accession number :
edsair.doi...........910f5260a14d59664d43964434b13b6f
Full Text :
https://doi.org/10.1103/physrevb.93.024304