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An investigation into the Brønsted acidity of the perfluorinated alkoxy silanes {(F3C)3CO}3SiH and {(F6C5)3CO}2Si(Cl)H

Authors :
Felix Feige
Lorraine A. Malaspina
Florian Kleemiss
Julius F. Kögel
Sergey Ketkov
Emanuel Hupf
Simon Grabowsky
Jens Beckmann
Source :
Dalton Transactions. 52:5918-5925
Publication Year :
2023
Publisher :
Royal Society of Chemistry (RSC), 2023.

Abstract

The Si–H bond in {(F3C)3CO}3SiH is exceptionally strong and short; yet the acidity is comparable to common organic acids. This apparent contradiction will be discussed with the aid of contemporary DFT methods.

Subjects

Subjects :
Inorganic Chemistry

Details

ISSN :
14779234 and 14779226
Volume :
52
Database :
OpenAIRE
Journal :
Dalton Transactions
Accession number :
edsair.doi...........848f66c0107c12f3b0a96cb983993bb7
Full Text :
https://doi.org/10.1039/d3dt00299c