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Independent Freezing of Charge and Spin Dynamics inLa1.5Sr0.5CoO4

Authors :
John Hill
Igor Zaliznyak
Yutaka Moritomo
R. W. Erwin
John M. Tranquada
Source :
Physical Review Letters. 85:4353-4356
Publication Year :
2000
Publisher :
American Physical Society (APS), 2000.

Abstract

We present elastic and quasielastic neutron scattering measurements characterizing peculiar short-range charge-orbital and spin order in the layered perovskite material La{sub 1.5}Sr {sub 0.5}CoO {sub 4} . We find that below T{sub c}{approx}750 K holes introduced by Sr doping lose mobility and enter a statically ordered charge glass phase with loosely correlated checkerboard arrangement of empty and occupied d{sub 3z{sup 2}-r{sup 2}} orbitals (Co{sup 3+} and Co{sup 2+} ). The dynamics of the resultant mixed spin system is governed by the anisotropic nature of the crystal-field Hamiltonian and the peculiar exchange pattern produced by the orbital order. It undergoes a spin freezing transition at a much lower temperature, T{sub s}{approx}

Details

ISSN :
10797114 and 00319007
Volume :
85
Database :
OpenAIRE
Journal :
Physical Review Letters
Accession number :
edsair.doi...........819a9bf77603ed7d306cbe0366f3a531
Full Text :
https://doi.org/10.1103/physrevlett.85.4353