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Highly efficient visible light driven photocatalytic activities of the LaCuS2-graphene composite-decorated ordered mesoporous silica

Authors :
Jung-Hun Woo
Kwang Youn Cho
Dinh Cung Tien Nguyen
Chong-Hun Jung
Won-Chun Oh
Source :
Separation and Purification Technology. 205:11-21
Publication Year :
2018
Publisher :
Elsevier BV, 2018.

Abstract

A combination of mesoporous silica with an LaCuS2-graphene composite has been prepared by a self-assembly method in support of the CTAB surfactant as the structure creator and basic medium. The characterization was investigated using XRD, SEM, TEM, HR-TEM, EDS, XPS, Raman, and DRS analysis. The pore size of the as-fabricated composite was calculated to be 5.83 nm by the nitrogen adsorption/desorption isotherms. In addition, the photocatalytic properties revealed that the mesoporous SiO2/LaCuS2-graphene catalyst presented a good result for the photocatalytic activity of organic dyes and gallic acid under visible light irradiation. Moreover, the as-prepared mesoporous SiO2/LaCuS2-graphene nanocomposite exhibited a good photodegradation rate for a cationic organic dye group under a pH medium of 11. The photocatalytic performance of the phenol compound representation presented a good result, and the optimum amount of the catalytic for the gallic acid photocatalytic activity is 0.05 g. In addition, the mesoporous SiO2/LaCuS2-graphene catalyst can be exploited for the application of solar energy conversion with high hydrogen production capacity.

Details

ISSN :
13835866
Volume :
205
Database :
OpenAIRE
Journal :
Separation and Purification Technology
Accession number :
edsair.doi...........7fcd9f5cb8c99a6e6bf9606301159857
Full Text :
https://doi.org/10.1016/j.seppur.2018.05.019