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α-Diimine synthesis via titanium-mediated multicomponent diimination of alkynes with C-nitrosos

Authors :
Connor W. Frye
Dominic T. Egger
Errikos Kounalis
Adam J. Pearce
Yukun Cheng
Ian A. Tonks
Source :
Chemical Science. 13:1469-1477
Publication Year :
2022
Publisher :
Royal Society of Chemistry (RSC), 2022.

Abstract

Alkyne diimination to unsymmetric α-diimines can be achieved via multicomponent reaction of Ti imidos and C-nitrosos. C-nitroso [4 + 2] cycloaddition across a diazatitanacyclohexadiene initiates cascading retrocycloadditions, liberating the α-diimine.

Subjects

Subjects :
General Chemistry

Details

ISSN :
20416539 and 20416520
Volume :
13
Database :
OpenAIRE
Journal :
Chemical Science
Accession number :
edsair.doi...........7f2ece9711da62f0b5faf78704976024