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Charge-gap formation in the insulating states ofAV10O15(A= Ba, Sr)

Authors :
Y. Tokura
T. Kanzaki
Masaki Uchida
Takuro Katsufuji
T. Kajita
M. Hoshino
Source :
Physical Review B. 85
Publication Year :
2012
Publisher :
American Physical Society (APS), 2012.

Abstract

We measured the optical conductivity spectra of SrV${}_{10}$O${}_{15}$ with V${}^{2.8+}$, which exhibits an insulating behavior without any phase transition, and compared the results with those of BaV${}_{10}$O${}_{15}$, which shows orbital ordering below ${T}_{c}=123$ K. We found that a soft gap opens at the lowest temperature but it collapses with increasing temperature in SrV${}_{10}$O${}_{15}$, in contrast to a finite charge gap ($\ensuremath{\sim}0.3$ eV) in BaV${}_{10}$O${}_{15}$ below ${T}_{c}$. We also found that the difference of the conductivity spectra between SrV${}_{10}$O${}_{15}$ and BaV${}_{10}$O${}_{15}$ evolves even above ${T}_{c}$ of Ba, indicating that the fluctuation of orbital ordering produces a pseudogap in BaV${}_{10}$O${}_{15}$.

Details

ISSN :
1550235X and 10980121
Volume :
85
Database :
OpenAIRE
Journal :
Physical Review B
Accession number :
edsair.doi...........6fd25223eadc1ea3a68d30c628a3f7a4