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Absolute measurement of thePu242neutron-capture cross section

Authors :
Brian Bucher
John M. O'Donnell
A. Chyzh
Marian Jandel
Bayarbadrakh Baramsai
J. L. Ullmann
Aaron Couture
Shea Mosby
Ching-Yen Wu
Roger Henderson
Todd Bredeweg
M. Q. Buckner
Source :
Physical Review C. 93
Publication Year :
2016
Publisher :
American Physical Society (APS), 2016.

Abstract

The absolute neutron-capture cross section of $^{242}\mathrm{Pu}$ was measured at the Los Alamos Neutron Science Center using the Detector for Advanced Neutron-Capture Experiments array along with a compact parallel-plate avalanche counter for fission-fragment detection. The first direct measurement of the $^{242}\mathrm{Pu}(n,\ensuremath{\gamma})$ cross section was made over the incident neutron energy range from thermal to $\ensuremath{\approx}6$ keV, and the absolute scale of the $(n,\ensuremath{\gamma})$ cross section was set according to the known $^{239}\mathrm{Pu}(n,f)$ resonance at ${E}_{n,R}=7.83$ eV. This was accomplished by adding a small quantity of $^{239}\mathrm{Pu}$ to the $^{242}\mathrm{Pu}$ sample. The relative scale of the cross section, with a range of four orders of magnitude, was determined for incident neutron energies from thermal to $\ensuremath{\approx}40$ keV. Our data, in general, are in agreement with previous measurements and those reported in ENDF/B-VII.1; the $^{242}\mathrm{Pu}(n,\ensuremath{\gamma})$ cross section at the ${E}_{n,R}=2.68$ eV resonance is within $2.4%$ of the evaluated value. However, discrepancies exist at higher energies; our data are $\ensuremath{\approx}30%$ lower than the evaluated data at ${E}_{n}\ensuremath{\approx}1$ keV and are approximately $2\ensuremath{\sigma}$ away from the previous measurement at ${E}_{n}\ensuremath{\approx}20$ keV.

Details

ISSN :
24699993 and 24699985
Volume :
93
Database :
OpenAIRE
Journal :
Physical Review C
Accession number :
edsair.doi...........56f24bc8ac8758f827482cb90a5287c0
Full Text :
https://doi.org/10.1103/physrevc.93.044613