Back to Search Start Over

Ultrasmall Moment Incommensurate Spin Density Wave Order Masking a Ferromagnetic Quantum Critical Point in NbFe2

Authors :
Enrico Faulhaber
F. M. Grosche
P. G. Niklowitz
A. Neubauer
Max Hirschberger
Christian Pfleiderer
Astrid Schneidewind
Petr Čermák
W. J. Duncan
Jean-Michel Mignot
M. Lucas
Source :
Physical Review Letters. 123
Publication Year :
2019
Publisher :
American Physical Society (APS), 2019.

Abstract

In the metallic magnet ${\mathrm{Nb}}_{1\ensuremath{-}y}{\mathrm{Fe}}_{2+y}$, the low temperature threshold of ferromagnetism can be investigated by varying the Fe excess $y$ within a narrow homogeneity range. We use elastic neutron scattering to track the evolution of magnetic order from Fe-rich, ferromagnetic ${\mathrm{Nb}}_{0.981}{\mathrm{Fe}}_{2.019}$ to approximately stoichiometric ${\mathrm{NbFe}}_{2}$, in which we can, for the first time, characterize a long-wavelength spin density wave state burying a ferromagnetic quantum critical point. The associated ordering wave vector ${\mathbf{q}}_{\mathrm{SDW}}=(0,0,{l}_{\mathrm{SDW}})$ is found to depend significantly on $y$ and $T$, staying finite but decreasing as the ferromagnetic state is approached. The phase diagram follows a two-order-parameter Landau theory, for which all of the coefficients can now be determined. Our findings suggest that the emergence of spin density wave order cannot be attributed to band structure effects alone. They indicate a common microscopic origin of both types of magnetic order and provide strong constraints on related theoretical scenarios based on, e.g., quantum order by disorder.

Details

ISSN :
10797114 and 00319007
Volume :
123
Database :
OpenAIRE
Journal :
Physical Review Letters
Accession number :
edsair.doi...........56c815f7b4fa746691327b1733a9e1f2
Full Text :
https://doi.org/10.1103/physrevlett.123.247203