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ABOVE THRESHOLD IONIZATION OF POLAR <font>NaK</font> MOLECULES DRIVEN BY FEW-CYCLE LASER PULSE
- Source :
- Journal of Theoretical and Computational Chemistry. :785-795
- Publication Year :
- 2010
- Publisher :
- World Scientific Pub Co Pte Lt, 2010.
-
Abstract
- We investigate theoretically the above-threshold ionization (ATI) of the polar NaK molecule exposed in few-cycle laser field by numerically solving the time-dependent Schrödinger equation including the vibrational and rotational degrees of freedom. The left and right ATI spectra are calculated by integrating the ionization continuum wave function over the left and the right half spheres along the laser polarization. We find that the left and right ATI spectra are asymmetric, and this asymmetry depends strongly on the molecular orientation and the carrier-envelope phase (CEP) of the laser pulse. Moreover, we also perform the calculation for different initially rotational states to study the effect of rotational temperature on the ATI dynamics.
- Subjects :
- Chemistry
Above threshold ionization
Carrier-envelope phase
Rotational temperature
Laser
Spectral line
Computer Science Applications
Schrödinger equation
law.invention
symbols.namesake
Computational Theory and Mathematics
law
Ionization
Physics::Atomic and Molecular Clusters
symbols
Physics::Atomic Physics
Physical and Theoretical Chemistry
Atomic physics
Wave function
Subjects
Details
- ISSN :
- 17936888 and 02196336
- Database :
- OpenAIRE
- Journal :
- Journal of Theoretical and Computational Chemistry
- Accession number :
- edsair.doi...........56350a2232e3af96c5b5cd22bf0708ff
- Full Text :
- https://doi.org/10.1142/s0219633610006018