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ABOVE THRESHOLD IONIZATION OF POLAR <font>NaK</font> MOLECULES DRIVEN BY FEW-CYCLE LASER PULSE

Authors :
Jie Yu
Shu-Lin Cong
Wen-Hui Hu
Chuan-Cun Shu
Source :
Journal of Theoretical and Computational Chemistry. :785-795
Publication Year :
2010
Publisher :
World Scientific Pub Co Pte Lt, 2010.

Abstract

We investigate theoretically the above-threshold ionization (ATI) of the polar NaK molecule exposed in few-cycle laser field by numerically solving the time-dependent Schr&#246;dinger equation including the vibrational and rotational degrees of freedom. The left and right ATI spectra are calculated by integrating the ionization continuum wave function over the left and the right half spheres along the laser polarization. We find that the left and right ATI spectra are asymmetric, and this asymmetry depends strongly on the molecular orientation and the carrier-envelope phase (CEP) of the laser pulse. Moreover, we also perform the calculation for different initially rotational states to study the effect of rotational temperature on the ATI dynamics.

Details

ISSN :
17936888 and 02196336
Database :
OpenAIRE
Journal :
Journal of Theoretical and Computational Chemistry
Accession number :
edsair.doi...........56350a2232e3af96c5b5cd22bf0708ff
Full Text :
https://doi.org/10.1142/s0219633610006018