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Zwitterionic complexes arising from the reaction of tucked-in titanocenes with tris(pentafluorophenyl)borane

Authors :
Jiří Kubišta
Ivana Císařová
Karel Mach
Vojtech Varga
Michal Horáček
Pavel Šindelář
Source :
Inorganic Chemistry Communications. 8:222-226
Publication Year :
2005
Publisher :
Elsevier BV, 2005.

Abstract

Single tucked-in titanocene [Ti(η5-C5Me5)(η5:η1-C5Me4CH2)] adds to B(C6F5)3 to give the paramagnetic cationic complex [Ti(η5-C5Me5){η5-C5Me4CH2B(C6F5)3}] (1). Doubly tucked-in titanocene [Ti(η5-C5Me5){η3:η4-C5Me3(CH2)2}] reacts with B(C6F5)3 by one methylene group to give [Ti(η5-C5Me5){η5:η1-C5Me3(CH2)CH2B(C6F5)3}] (6). The crystal structure of 6 revealed that one hydrogen of the methylene group attached to boron agostically interacts with Ti(IV).

Details

ISSN :
13877003
Volume :
8
Database :
OpenAIRE
Journal :
Inorganic Chemistry Communications
Accession number :
edsair.doi...........3ca4e702213ad0092c6c9f4f5387c1bc
Full Text :
https://doi.org/10.1016/j.inoche.2004.12.011